2007年6月
Spin-lattice instability to a fractional magnetization state in the spinel HgCr2O4
NATURE PHYSICS
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- 巻
- 3
- 号
- 6
- 開始ページ
- 397
- 終了ページ
- 400
- 記述言語
- 英語
- 掲載種別
- 研究論文(学術雑誌)
- DOI
- 10.1038/nphys586
- 出版者・発行元
- NATURE PUBLISHING GROUP
Magnetic systems are fertile ground for the emergence of exotic states(1) when the magnetic interactions cannot be satisfied simultaneously owing to the topology of the lattice - a situation known as geometrical frustration(2,3). Spinels, AB(2)O(4), can realize the most highly frustrated network of corner-sharing tetrahedra(1-3). Several novel states have been discovered in spinels, such as composite spin clusters(1) and novel charge-ordered states(4-6). Here, we use neutron and synchrotron X-ray scattering to characterize the fractional magnetization state of HgCr2O4 under an external magnetic field, H. When the field is applied in its Neel ground state, a phase transition occurs at H similar to 10 T at which each tetrahedron changes from a canted Neel state to a fractional spin state with the total spin, S-tet, of S/2 and the lattice undergoes an orthorhombic to cubic symmetry change. Our results provide the microscopic one-to-one correspondence between the spin state and the lattice distortion.
- リンク情報
- ID情報
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- DOI : 10.1038/nphys586
- ISSN : 1745-2473
- Web of Science ID : WOS:000247344400014