論文

査読有り
2019年5月

Planar Perovskite Solar Cells with High Efficiency and Fill Factor Obtained Using Two-Step Growth Process

ACS APPLIED MATERIALS & INTERFACES
  • Fengjiu Yang
  • ,
  • Jiewei Liu
  • ,
  • Xiaofan Wang
  • ,
  • Kenya Tanaka
  • ,
  • Keisuke Shinokita
  • ,
  • Yuhei Miyauchi
  • ,
  • Atsushi Wakamiya
  • ,
  • Kazunari Matsuda

11
17
開始ページ
15680
終了ページ
15687
記述言語
英語
掲載種別
研究論文(学術雑誌)
DOI
10.1021/acsami.9b02948
出版者・発行元
AMER CHEMICAL SOC

Hybrid organic inorganic perovskite solar cells (PSCs) have been regarded as the most promising next-generation photovoltaics (PVs) because of their potential for low-cost fabrication and advances in their development. Superior quality of the photoactive perovskite layer is a main factor for further increasing the PV performance of the organic inorganic perovskite solar cells (PSCs). Herein, we successfully obtained perovskite with a high crystallinity and large grain size by utilizing excess PbI2 and SSGP technique and demonstrated a superior PV performance of normal-architecture planar PSCs. The SSGP PSCs with the highest fill factor (FF) reported thus far (83.4%) to our knowledge were obtained without sacrificing other PV parameters. Moreover, a high efficiency of 21.3% (21.6%) with a high FF of 80.0% (81.2%) in forward (reverse) scan was achieved. The unencapsulated SSGP PSCs showed robust continuous light-soaking and thermal stability under harsh characterization conditions. Additionally, we achieved a high efficiency of 20.1% with a negligible hysteresis on the large active area SSGP PSCs (similar to 1 cm(2)). The optical properties, efficient carrier extraction, and reduction of recombination loss of the SSGP perovskite significantly contribute to the high PV performance and robust stability of SSGP PSCs.

リンク情報
DOI
https://doi.org/10.1021/acsami.9b02948
Web of Science
https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=JSTA_CEL&SrcApp=J_Gate_JST&DestLinkType=FullRecord&KeyUT=WOS:000466988800054&DestApp=WOS_CPL
ID情報
  • DOI : 10.1021/acsami.9b02948
  • ISSN : 1944-8244
  • eISSN : 1944-8252
  • Web of Science ID : WOS:000466988800054

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