論文

2021年9月13日

Radiative lifetime and dynamics of trions in few-layered ReS2

Applied Physics Letters
  • Xiaofan Wang
  • ,
  • Keisuke Shinokita
  • ,
  • Kazunari Matsuda

119
11
開始ページ
113103
終了ページ
113103
記述言語
英語
掲載種別
研究論文(学術雑誌)
DOI
10.1063/5.0059198
出版者・発行元
AIP Publishing

Few-layered ReS2 with anisotropic electrical and optical properties has attracted much attention in the research field of two-dimensional (2D) materials. Recently, a stable charged exciton (trion) composed of bound states of two electrons and a hole with large binding energy has been experimentally observed in a few-layered ReS2. However, the dynamics of stable trions remain unclear. We studied the excited-state dynamics, including the radiative lifetime of the negative trion in three layer (3L)-ReS2 via temperature-dependent photoluminescence spectroscopy and phenomenological rate-equation analysis. The derived radiative lifetime of the trion increases linearly with increasing temperature, reaching a few nanoseconds at a high temperature of 150 K; this observation implies that the experimentally observed negative trion in 3L-ReS2 lies in the optically allowed state. Our results provide significant insights into the physics of excitonic states in 2D materials. Published under an exclusive license by AIP Publishing.

リンク情報
DOI
https://doi.org/10.1063/5.0059198
Web of Science
https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=JSTA_CEL&SrcApp=J_Gate_JST&DestLinkType=FullRecord&KeyUT=WOS:000724314700006&DestApp=WOS_CPL
URL
https://aip.scitation.org/doi/pdf/10.1063/5.0059198
ID情報
  • DOI : 10.1063/5.0059198
  • ISSN : 0003-6951
  • eISSN : 1077-3118
  • Web of Science ID : WOS:000724314700006

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