論文

査読有り
2014年3月18日

A new metric for long-range transport potential of chemicals

Environmental Science and Technology
  • Toru Kawai
  • ,
  • Karolina Jagiello
  • ,
  • Anita Sosnowska
  • ,
  • Katarzyna Odziomek
  • ,
  • Agnieszka Gajewicz
  • ,
  • Itsuki C. Handoh
  • ,
  • Tomasz Puzyn
  • ,
  • Noriyuki Suzuki

48
6
開始ページ
3245
終了ページ
3252
記述言語
英語
掲載種別
研究論文(学術雑誌)
DOI
10.1021/es4026003
出版者・発行元
AMER CHEMICAL SOC

We propose a new metric for long-range transport potential (LRTP), GIF, based on source-receptor analyses and evaluate the LRTP and persistence of a wide variety of chlorinated and brominated organic compounds using GIF and overall persistence (POV), respectively. We calculated GIF and P OV using our global 3D dynamic multimedia model (FATE). Physicochemical properties were obtained from quantitative structure-property relationship (QSPR) models. The FATE-QSPR combined model enabled us to systematically investigate the LRTP and persistence of a wide variety of chemical substances. On average, the estimated GIF and POV for chlorinated compounds were larger than those for their brominated counterparts, with the largest and smallest values found for polychlorinated biphenyls and polybrominated dibenzodioxins, respectively. We also compared GIF with four differently defined LRTP metrics and two LRTP metrics obtained from a simple model. The results of our analyses indicate that the LRTP ranks can differ considerably among LRTP metrics, the differences being dependent on the governing environmental processes, relevant physicochemical properties, and multimedia model. © 2014 American Chemical Society.

リンク情報
DOI
https://doi.org/10.1021/es4026003
PubMed
https://www.ncbi.nlm.nih.gov/pubmed/24579696
Web of Science
https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=JSTA_CEL&SrcApp=J_Gate_JST&DestLinkType=FullRecord&KeyUT=WOS:000333776000021&DestApp=WOS_CPL
Scopus
https://www.scopus.com/inward/record.uri?partnerID=HzOxMe3b&scp=84898986959&origin=inward
Scopus Citedby
https://www.scopus.com/inward/citedby.uri?partnerID=HzOxMe3b&scp=84898986959&origin=inward
ID情報
  • DOI : 10.1021/es4026003
  • ISSN : 0013-936X
  • eISSN : 1520-5851
  • PubMed ID : 24579696
  • SCOPUS ID : 84898986959
  • Web of Science ID : WOS:000333776000021

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