論文

国際誌
2021年5月21日

Strong spin-orbit coupling inducing Autler-Townes effect in lead halide perovskite nanocrystals.

Nature communications
  • Go Yumoto
  • ,
  • Hideki Hirori
  • ,
  • Fumiya Sekiguchi
  • ,
  • Ryota Sato
  • ,
  • Masaki Saruyama
  • ,
  • Toshiharu Teranishi
  • ,
  • Yoshihiko Kanemitsu

12
1
開始ページ
3026
終了ページ
3026
記述言語
英語
掲載種別
研究論文(学術雑誌)
DOI
10.1038/s41467-021-23291-w

Manipulation of excitons via coherent light-matter interaction is a promising approach for quantum state engineering and ultrafast optical modulation. Various excitation pathways in the excitonic multilevel systems provide controllability more efficient than that in the two-level system. However, these control schemes have been restricted to limited control-light wavelengths and cryogenic temperatures. Here, we report that lead halide perovskites can lift these restrictions owing to their multiband structure induced by strong spin-orbit coupling. Using CsPbBr3 perovskite nanocrystals, we observe an anomalous enhancement of the exciton energy shift at room temperature with increasing control-light wavelength from the visible to near-infrared region. The enhancement occurs because the interconduction band transitions between spin-orbit split states have large dipole moments and induce a crossover from the two-level optical Stark effect to the three-level Autler-Townes effect. Our finding establishes a basis for efficient coherent optical manipulation of excitons utilizing energy states with large spin-orbit splitting.

リンク情報
DOI
https://doi.org/10.1038/s41467-021-23291-w
PubMed
https://www.ncbi.nlm.nih.gov/pubmed/34021150
ID情報
  • DOI : 10.1038/s41467-021-23291-w
  • PubMed ID : 34021150

エクスポート
BibTeX RIS