論文

査読有り 筆頭著者 責任著者
2020年11月

Kinetic-model-based design of industrial reactor for catalytic hydrogen production via ammonia decomposition

Chemical Engineering Research and Design
  • Atsushi Takahashi
  • ,
  • Tadahiro Fujitani

165
開始ページ
333
終了ページ
340
記述言語
英語
掲載種別
研究論文(学術雑誌)
DOI
10.1016/j.cherd.2020.11.004
出版者・発行元
Elsevier BV

A two-dimensional reactor model based on reaction kinetics and heat and mass transfer for catalytic NH3 decomposition was constructed. A reactor design that minimizes the effect of endothermic reaction was investigated. It is difficult to design a single-tube reactor for NH3 treatment at a flow rate of 10 m(3)/h because heat transfer from the reactor wall cannot keep up with the fast consumption of heat by the reaction, even under low space velocity conditions. The target conversion was achieved by decreasing the NH3 supply rate. A reactor with a packed bed of suitable length was designed. Industrial-scale NH3 treatment can be achieved using a multi-tube reactor. (C) 2020 Institution of Chemical Engineers. Published by Elsevier B.V. All rights reserved.

リンク情報
DOI
https://doi.org/10.1016/j.cherd.2020.11.004
Web of Science
https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=JSTA_CEL&SrcApp=J_Gate_JST&DestLinkType=FullRecord&KeyUT=WOS:000615860900006&DestApp=WOS_CPL
ID情報
  • DOI : 10.1016/j.cherd.2020.11.004
  • ISSN : 0263-8762
  • eISSN : 1744-3563
  • Web of Science ID : WOS:000615860900006

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