This paper examines a new method for evaluating the stability of rock blocks on slopes using a remotely positioned Laser Doppler Vibrometer (LDV). A series of experiments using physical models were conducted to evaluate the validity of this new method. Based on the experimental studies, the applicability of LDV was examined by comparing results with a conventional seismometer measurement. To examine the quantitative correlations between vibration properties and the stability of a rock block, the effects on the vibration properties of the size of the rock block, the initial block position, the slope incline, and the type of ground surface were studied. The experimental results showed that LDV measurements agreed with conventional seismometer measurements. There was also a good correlation between vibration properties and rock-block stability. On the other hand, it was found that for a boulder on tightly compacted ground, the application of block stability assessment by tonometry was difficult when measuring microtremors or sloppy vibration due to nearby vehicle traffic. Furthermore, numerical analysis of the slope model was carried out to examine the validity of the model experiment and application of the suggested technique. The results of the analysis demonstrated that the suggested technique was effective for application to stability monitoring of a block and evaluation of the effect of stability measures.