論文

査読有り 国際共著
2020年1月

Influence of nonequilibrium phonons on the spin dynamics of a single Cr atom

Physical Review B
  • V., Tiwari
  • ,
  • K., Makita
  • ,
  • M., Arino
  • ,
  • M., Morita
  • ,
  • 黒田, 眞司
  • ,
  • H., Boukari
  • ,
  • L
  • ,
  • Besombes

101
3
開始ページ
035305
終了ページ
記述言語
日本語
掲載種別
研究論文(学術雑誌)
DOI
10.1103/PhysRevB.101.035305
出版者・発行元
American Physical Society

We analyze the influence of optically generated nonequilibrium phonons on the spin relaxation and effective spin temperature of an individual Cr atom inserted in a quantum dot. Using a three-pulse pump-probe technique, we show that the spin relaxation measured in resonant optical pumping experiments strongly depends on the optical excitation conditions. We observe for an isolated Cr in the dark a heating time shorter than a few hundred nanoseconds after an initial high-power nonresonant excitation pulse. A cooling time larger than a few tens of microseconds, independent of the excitation, is obtained in the same experimental conditions. We show that a tunable spin-lattice coupling dependent on the density of nonequilibrium phonons can explain the observed dynamics. Low-energy excitation conditions are found where the Cr spin states S-z = +/- 1 can be efficiently populated by a nonresonant optical excitation, prepared and read out by resonant optical pumping and conserved in the dark for a few microseconds.

リンク情報
DOI
https://doi.org/10.1103/PhysRevB.101.035305
ID情報
  • DOI : 10.1103/PhysRevB.101.035305
  • ISSN : 2469-9950

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