論文

査読有り 国際共著
2020年7月22日

Effect of Nd and Rh substitution on the spin dynamics of the Kondo-insulator CeFe2Al10

PHYSICAL REVIEW B
  • Alekseev, P. A.
  • ,
  • Mignot, J-M
  • ,
  • Adroja, D. T.
  • ,
  • Lazukov, V. N.
  • ,
  • Tanida, H.
  • ,
  • Muro, Y.
  • ,
  • Sera, M.
  • ,
  • Takabatake, T.
  • ,
  • Steffens, P.
  • ,
  • Rols, S.

102
2
DOI
10.1103/PhysRevB.102.024438
出版者・発行元
AMER PHYSICAL SOC

The dynamic magnetic properties of the Kondo-insulator state in CeFe2Al10 (spin gap, resonance mode) have been investigated using polarized neutrons on a single crystal of pure CeFe2Al10 . The results indicate that the magnetic excitations are polarized mainly along the orthorhombic a axis and their dispersion along the orthorhombic c direction could be determined. Polycrystalline samples of Nd- and Rh-doped CeFe2Al10 were also studied by the time-of-flight technique, with the aim of finding out how the low-energy magnetic excitation spectra change upon isoelectronic substitution of a rare-earth element (Nd) on the magnetic Ce site or electron doping (Rh) on the transition-element Fe sublattice. The introduction of magnetic Nd impurities strongly modifies the spin gap in the Ce dynamic magnetic response and causes the appearance of a quasielastic signal. The crystal-field excitations of Nd, studied in both LaFe2Al10 and CeFe2Al10, also reveal a significant influence of f -electron hybridization (largest in the case of Ce) on the crystal-field potential. As a function of the Rh concentration, a gradual change is observed from a Kondo-insulator to a metallic Kondo-lattice response, likely reflecting the decrease in the hybridization energy.

リンク情報
DOI
https://doi.org/10.1103/PhysRevB.102.024438
ID情報
  • DOI : 10.1103/PhysRevB.102.024438
  • ISSN : 2469-9950

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