論文

査読有り
2022年7月29日

Rapidly expanding spin-polarized exciton halo in a two-dimensional halide perovskite at room temperature

Science Advances
  • Go Yumoto
  • ,
  • Fumiya Sekiguchi
  • ,
  • Ruito Hashimoto
  • ,
  • Tomoya Nakamura
  • ,
  • Atsushi Wakamiya
  • ,
  • Yoshihiko Kanemitsu

8
30
開始ページ
abp8135
終了ページ
記述言語
掲載種別
研究論文(学術雑誌)
DOI
10.1126/sciadv.abp8135
出版者・発行元
American Association for the Advancement of Science (AAAS)

Monitoring of the spatially resolved exciton spin dynamics in two-dimensional semiconductors has revealed the formation of a spatial pattern and long-range transport of the spin-polarized excitons, which holds promise for exciton-based spin-optoelectronic applications. However, the spatial evolution has been restricted to cryogenic temperatures because of the short exciton spin relaxation times at room temperature. Here, we report that two-dimensional halide perovskites can overcome this limitation owing to their relatively long exciton spin relaxation times and substantial exciton-exciton interactions. We demonstrate the emergence of a halo-like spatial profile in spin-polarized exciton population and its ultrafast expansion at room temperature by performing time-resolved Faraday rotation imaging of spin-polarized excitons in two-dimensional perovskite (C 4 H 9 NH 3 ) 2 (CH 3 NH 3 ) 3 Pb 4 I 13 . Exciton-exciton exchange interactions induce density-dependent nonlinear relaxation and ultrafast transport of exciton spins and give rise to a rapidly expanding halo-like spatial pattern. The density-dependent spatial control suggests the potential of using two-dimensional halide perovskites for spin-optoelectronic applications.

リンク情報
DOI
https://doi.org/10.1126/sciadv.abp8135
ID情報
  • DOI : 10.1126/sciadv.abp8135
  • eISSN : 2375-2548

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