Papers

Peer-reviewed
Jun, 2010

Evidence for a Correlated Insulator to Antiferromagnetic Metal Transition in CrN

PHYSICAL REVIEW LETTERS
  • P. A. Bhobe
  • A. Chainani
  • M. Taguchi
  • T. Takeuchi
  • R. Eguchi
  • M. Matsunami
  • K. Ishizaka
  • Y. Takata
  • M. Oura
  • Y. Senba
  • H. Ohashi
  • Y. Nishino
  • M. Yabashi
  • K. Tamasaku
  • T. Ishikawa
  • K. Takenaka
  • H. Takagi
  • S. Shin
  • Display all

Volume
104
Number
23
Language
English
Publishing type
Research paper (scientific journal)
DOI
10.1103/PhysRevLett.104.236404
Publisher
AMER PHYSICAL SOC

We investigate the electronic structure of chromium nitride (CrN) across the first-order magneto-structural transition at T-N similar to 286 K. Resonant photoemission spectroscopy (PES) shows a gap in the 3d partial density of states at the Fermi level and an on-site Coulomb energy U similar to 4.5 eV, indicating strong electron-electron correlations. Bulk-sensitive high-resolution (6 meV) laser PES reveals a clear Fermi edge indicating an antiferromagnetic metal below T-N. Hard x-ray Cr 2p core-level PES shows T-dependent changes across T-N which originate from screening due to coherent states as substantiated by cluster model calculations using the experimentally observed U. Electrical resistivity confirms an insulator above T-N (E-g similar to 70 meV) becoming a disordered metal below T-N. Thus, CrN transforms from a correlated insulator to an antiferromagnetic metal, coupled to the magnetostructural transition.

Link information
DOI
https://doi.org/10.1103/PhysRevLett.104.236404
Web of Science
https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=JSTA_CEL&SrcApp=J_Gate_JST&DestLinkType=FullRecord&KeyUT=WOS:000278658500002&DestApp=WOS_CPL
ID information
  • DOI : 10.1103/PhysRevLett.104.236404
  • ISSN : 0031-9007
  • Web of Science ID : WOS:000278658500002

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