論文

査読有り
2007年10月

Electronic structure of LaNiO(3-x): An in situ soft x-ray photoemission and absorption study

PHYSICAL REVIEW B
  • K. Horiba
  • ,
  • R. Eguchi
  • ,
  • M. Taguchi
  • ,
  • A. Chainani
  • ,
  • A. Kikkawa
  • ,
  • Y. Senba
  • ,
  • H. Ohashi
  • ,
  • S. Shin

76
15
記述言語
英語
掲載種別
研究論文(学術雑誌)
DOI
10.1103/PhysRevB.76.155104
出版者・発行元
AMER PHYSICAL SOC

We study the electronic structure of LaNiO(3-x) thin films using in situ soft x-ray photoemission and absorption spectroscopy. The in situ high-resolution measurements reveal that states at and near the Fermi level (E(F)) in the occupied and unoccupied densities of states are very sensitive to the oxygen content and are directly related to a metal-insulator transition. The highest quality epitaxial films of LaNiO(3) show a temperature-dependent sharp peak at E(F). A detailed analysis of its electrical resistivity confirms a T(1.5) behavior over a large temperature range, which has been observed in earlier studies. Local density approximation band structure calculations indicate that the narrowing of the Ni d e(g) electron derived peak at E(F) cannot be reproduced by a strained crystal structure, suggesting a renormalization of electronic states at E(F) in LaNiO(3). The T-dependent spectral changes at E(F), coupled with the resistivity behavior and proximity to a metal-insulator transition, suggest the role of electron correlations in LaNiO(3).

リンク情報
DOI
https://doi.org/10.1103/PhysRevB.76.155104
Web of Science
https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=JSTA_CEL&SrcApp=J_Gate_JST&DestLinkType=FullRecord&KeyUT=WOS:000250620400036&DestApp=WOS_CPL
ID情報
  • DOI : 10.1103/PhysRevB.76.155104
  • ISSN : 1098-0121
  • Web of Science ID : WOS:000250620400036

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