論文

査読有り 国際誌
2021年2月16日

Enhancing the Hot-Phonon Bottleneck Effect in a Metal Halide Perovskite by Terahertz Phonon Excitation

Physical Review Letters
  • Fumiya Sekiguchi
  • ,
  • Hideki Hirori
  • ,
  • Go Yumoto
  • ,
  • Ai Shimazaki
  • ,
  • Tomoya Nakamura
  • ,
  • Atsushi Wakamiya
  • ,
  • Yoshihiko Kanemitsu

126
7
開始ページ
077401
終了ページ
077401
記述言語
英語
掲載種別
研究論文(学術雑誌)
DOI
10.1103/physrevlett.126.077401
出版者・発行元
American Physical Society (APS)

We investigate the impact of phonon excitations on the photoexcited carrier dynamics in a lead-halide perovskite CH_{3}NH_{3}PbI_{3}, which hosts unique low-energy phonons that can be directly excited by terahertz pulses. Our time-resolved photoluminescence measurements reveal that strong terahertz excitation prolongs the cooling time of hot carriers, providing direct evidence for the hot-phonon bottleneck effect. In contrast to the previous studies where phonons are treated as a passive heat bath, our results demonstrate that phonon excitation can significantly perturb the carrier relaxation dynamics in halide perovskites through the coupling between transverse- and longitudinal-optical phonons.

リンク情報
DOI
https://doi.org/10.1103/physrevlett.126.077401
PubMed
https://www.ncbi.nlm.nih.gov/pubmed/33666485
URL
https://link.aps.org/article/10.1103/PhysRevLett.126.077401
URL
http://harvest.aps.org/v2/journals/articles/10.1103/PhysRevLett.126.077401/fulltext
ID情報
  • DOI : 10.1103/physrevlett.126.077401
  • ISSN : 0031-9007
  • eISSN : 1079-7114
  • PubMed ID : 33666485

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