論文

査読有り
2014年3月

Bulk nature of layered perovskite iridates beyond the Mott scenario: An approach from a bulk-sensitive photoemission study

PHYSICAL REVIEW B
  • A. Yamasaki
  • S. Tachibana
  • H. Fujiwara
  • A. Higashiya
  • A. Irizawa
  • O. Kirilmaz
  • F. Pfaff
  • P. Scheiderer
  • J. Gabel
  • M. Sing
  • T. Muro
  • M. Yabashi
  • K. Tamasaku
  • H. Sato
  • H. Namatame
  • M. Taniguchi
  • A. Hloskovskyy
  • H. Yoshida
  • H. Okabe
  • M. Isobe
  • J. Akimitsu
  • W. Drube
  • R. Claessen
  • T. Ishikawa
  • S. Imada
  • A. Sekiyama
  • S. Suga
  • 全て表示

89
12
開始ページ
121111(R)/1
終了ページ
5
記述言語
英語
掲載種別
研究論文(学術雑誌)
DOI
10.1103/PhysRevB.89.121111
出版者・発行元
AMER PHYSICAL SOC

We present genuine bulk Ir 5d j(eff) states of layered perovskite iridates obtained by hard-x-ray photoemission spectroscopy (HAXPES) with s- and p-polarized lights. HAXPES spectra of Sr2IrO4 and Ba2IrO4 are well reproduced by the quasiparticle density of states calculated by the local density approximation with dynamical mean-field theory (LDA + DMFT). It is demonstrated that the insulating nature of the iridates is triggered by antiferromagnetic correlation (Slater type) combined with electron correlation (Mott type). The extremely-lowenergy bulk-sensitive photoemission spectroscopy reveals "bad metallic" states in the paramagnetic phase of the iridates, suggesting strongly renormalized metallic states above the Neel temperature as predicted by the LDA + DMFT.

リンク情報
DOI
https://doi.org/10.1103/PhysRevB.89.121111
Web of Science
https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=JSTA_CEL&SrcApp=J_Gate_JST&DestLinkType=FullRecord&KeyUT=WOS:000333239700001&DestApp=WOS_CPL
ID情報
  • DOI : 10.1103/PhysRevB.89.121111
  • ISSN : 1098-0121
  • eISSN : 1550-235X
  • Web of Science ID : WOS:000333239700001

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