論文

2022年2月1日

Contrasting magnetic structures in SrLaCuSbO6 and SrLaCuNbO6: Spin- 12 quasi-square-lattice J1-J2 Heisenberg antiferromagnets

Physical Review B
  • Masari Watanabe
  • ,
  • Nobuyuki Kurita
  • ,
  • Hidekazu Tanaka
  • ,
  • Wataru Ueno
  • ,
  • Kazuki Matsui
  • ,
  • Takayuki Goto
  • ,
  • Masato Hagihala

105
5
記述言語
掲載種別
研究論文(学術雑誌)
DOI
10.1103/PhysRevB.105.054414

We report the magnetic properties of the double perovskites SrLaCuSbO6 (SLCSO) and SrLaCuNbO6 (SLCNO). The temperature dependence of the magnetic susceptibilities of both compounds shows a broad maximum characteristic of an S=1/2 square lattice Heisenberg antiferromagnet. Magnetic ordering occurs at TN=13.6 and 15.7 K for SLCSO and SLCNO, respectively. Neutron powder diffraction measurements reveal contrasting spin structures in both compounds. The spin structures of SLCSO and SLCNO below TN are Néel antiferromagnetic and columnar antiferromagnetic, respectively. This result demonstrates that the nearest-neighbor interaction is dominant in SLCSO, whereas the next-nearest-neighbor interaction is dominant in SLCNO. The magnitude of the ordered moment was evaluated at 3.5 K to be m=0.39(3)μB for SLCSO and 0.37(1)μB for SLCNO, which are significantly smaller than those calculated using linear spin wave theory. We infer that the small ordered moment is caused by the effect of bond randomness arising from the site disorder of Sr and La ions.

リンク情報
DOI
https://doi.org/10.1103/PhysRevB.105.054414
Scopus
https://www.scopus.com/inward/record.uri?partnerID=HzOxMe3b&scp=85125204616&origin=inward
Scopus Citedby
https://www.scopus.com/inward/citedby.uri?partnerID=HzOxMe3b&scp=85125204616&origin=inward
ID情報
  • DOI : 10.1103/PhysRevB.105.054414
  • ISSN : 2469-9950
  • eISSN : 2469-9969
  • SCOPUS ID : 85125204616

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