Papers

May, 2015

Characterization of the magnetic moment distribution in low-concentration solutions of iron oxide nanoparticles by a high-T-c superconducting quantum interference device magnetometer

JOURNAL OF APPLIED PHYSICS
  • M. M. Saari
  • ,
  • K. Sakai
  • ,
  • T. Kiwa
  • ,
  • T. Sasayama
  • ,
  • T. Yoshida
  • ,
  • K. Tsukada

Volume
117
Number
17
Language
English
Publishing type
Research paper (scientific journal)
DOI
10.1063/1.4919043
Publisher
AMER INST PHYSICS

We developed a highly sensitive AC/DC magnetometer using a high-temperature superconductor superconducting quantum interference device for the evaluation of magnetic nanoparticles in solutions. Using the developed system, we investigated the distribution of magnetic moments of iron oxide multi-core particles of 100 nm at various iron concentrations that are lower than 96 mu g/ml by analyzing the measured magnetization curves. Singular value decomposition and non-regularized non-negative least-squares methods were used during the reconstruction of the distribution. Similar distributions were obtained for all concentrations, and the iron concentration could be determined from the measured magnetization curves. The measured harmonics upon the excitation of AC and DC magnetic fields curves agreed well with the harmonics simulated based on the reconstructed magnetization curves, implying that the magnetization curves of magnetic nanoparticles were successfully obtained as we will show in the article. We compared the magnetization curves between multi-core particles of 100 nm and 130 nm, composed of 12-nm iron oxide nanoparticles. A distinctive magnetic property between the 100 nm and 130 nm particles in low-concentration solutions was successfully characterized. The distribution characteristic of magnetic moments suggests that the net magnetic moment in a multi-core particle is affected by the size of the magnetic cores and their degree of aggregation. Exploration of magnetic properties with high sensitivity can be expected using the developed system. (C) 2015 AIP Publishing LLC.

Link information
DOI
https://doi.org/10.1063/1.4919043
Web of Science
https://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=JSTA_CEL&SrcApp=J_Gate_JST&DestLinkType=FullRecord&KeyUT=WOS:000354984100145&DestApp=WOS_CPL
ID information
  • DOI : 10.1063/1.4919043
  • ISSN : 0021-8979
  • eISSN : 1089-7550
  • Web of Science ID : WOS:000354984100145

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