論文

査読有り
2022年5月15日

Evolution of the electronic structure and correlations accompanied by suppression of itinerant ferromagnetism in Sr1-x(La0.5K0.5)xRuO3

Physical Review B
  • Ikuto Kawasaki
  • ,
  • Shin Ichi Fujimori
  • ,
  • Yukiharu Takeda
  • ,
  • Hiroshi Yamagami
  • ,
  • Rahmanto
  • ,
  • Yutoku Honma
  • ,
  • Kensuke Matsuoka
  • ,
  • Makoto Yokoyama

105
19
開始ページ
195122
終了ページ
記述言語
掲載種別
研究論文(学術雑誌)
DOI
10.1103/PhysRevB.105.195122

We have carried out soft x-ray photoemission experiments on itinerant ferromagnet Sr1-x(La0.5K0.5)xRuO3 to investigate how the electronic state varies with doping concentration. The Ru 4d-derived coherent part of the valence spectra develops significantly with increasing x for x≤0.3, which can be explained by the suppression of the ferromagnetic exchange splitting. With further increasing x, this development is overwhelmed by the spectral weight transfer from the coherent to the incoherent parts due to the electron correlation. The enhancement of the electron correlation effect with doping is also confirmed by the Ru 3d core-level spectra as the suppression of the well-screened peak. In contrast to the remarkable variation of the Ru 4d spectral intensity as a function of x, the valence spectra hardly depend on temperature and do not show any noticeable change across the magnetic transition temperatures, indicating that the temperature dependence of the exchange splitting cannot be explained by a simple Stoner picture. We compare the present photoemission results with those for isostructural Sr1-xAxRuO3 (A=La and Ca) and discuss the origin of the difference in the magnetic property between these doped compounds.

リンク情報
DOI
https://doi.org/10.1103/PhysRevB.105.195122
Scopus
https://www.scopus.com/inward/record.uri?partnerID=HzOxMe3b&scp=85131325685&origin=inward
Scopus Citedby
https://www.scopus.com/inward/citedby.uri?partnerID=HzOxMe3b&scp=85131325685&origin=inward
ID情報
  • DOI : 10.1103/PhysRevB.105.195122
  • ISSN : 2469-9950
  • eISSN : 2469-9969
  • SCOPUS ID : 85131325685

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