論文

査読有り
2020年11月2日

Impact of the Lattice on Magnetic Properties and Possible Spin Nematicity in the S=1 Triangular Antiferromagnet NiGa2S4

Physical Review Letters
  • Michael E. Valentine
  • ,
  • Tomoya Higo
  • ,
  • Yusuke Nambu
  • ,
  • Dipanjan Chaudhuri
  • ,
  • Jiajia Wen
  • ,
  • Collin Broholm
  • ,
  • Satoru Nakatsuji
  • ,
  • Natalia Drichko

125
19
開始ページ
197201
終了ページ
記述言語
掲載種別
研究論文(学術雑誌)
DOI
10.1103/PhysRevLett.125.197201

© 2020 American Physical Society. NiGa2S4 is a triangular lattice S=1 system with strong two dimensionality of the lattice, actively discussed as a candidate to host spin-nematic order brought about by strong quadrupole coupling. Using Raman scattering spectroscopy we identify a phonon of Eg symmetry which can modulate magnetic exchange J1 and produce quadrupole coupling. Additionally, our Raman scattering results demonstrate a loss of local inversion symmetry on cooling, which we associate with sulfur vacancies. This will lead to disordered Dzyaloshinskii-Moriya interactions, which can prevent long-range magnetic order. Using magnetic Raman scattering response we identify 160 K as a temperature of an upturn of magnetic correlations. The temperature range below 160 K, but above 50 K where antiferromagnetic correlations start to increase, is a candidate for spin-nematic regime.

リンク情報
DOI
https://doi.org/10.1103/PhysRevLett.125.197201
PubMed
https://www.ncbi.nlm.nih.gov/pubmed/33216581
Scopus
https://www.scopus.com/inward/record.uri?partnerID=HzOxMe3b&scp=85096094369&origin=inward
Scopus Citedby
https://www.scopus.com/inward/citedby.uri?partnerID=HzOxMe3b&scp=85096094369&origin=inward
ID情報
  • DOI : 10.1103/PhysRevLett.125.197201
  • ISSN : 0031-9007
  • eISSN : 1079-7114
  • PubMed ID : 33216581
  • SCOPUS ID : 85096094369

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