Jul, 2013
Quadrupole effects in tetragonal crystals PrCu2Si2 and DyCu2Si2
JOURNAL OF PHYSICS-CONDENSED MATTER
- Volume
- 25
- Number
- 29
- Language
- English
- Publishing type
- Research paper (scientific journal)
- DOI
- 10.1088/0953-8984/25/29/296002
- Publisher
- IOP PUBLISHING LTD
We have investigated quadrupole effects in tetragonal crystals of PrCu2Si2 and DyCu2Si2 by means of low-temperature ultrasonic measurements. The elastic constant C-44 of PrCu2Si2 exhibits pronounced softening below 70 K down to a Neel temperature T-N = 20 K, which is described in terms of a quadrupole susceptibility for a Gamma(5) doublet ground state and a Gamma(3) singlet first excited state located at 15.6 K in the crystalline electric field scheme. The C-44 and C-66 of DyCu2Si2 also show softening below 70 K down to T-N1 = 9.7 K. A low-lying pseudo-sextet state consisting of three Kramers doublets of Gamma(6) circle plus 2 Gamma(7) brings about softening of C-44 and C-66 in DyCu2Si2.
- Link information
- ID information
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- DOI : 10.1088/0953-8984/25/29/296002
- ISSN : 0953-8984
- eISSN : 1361-648X
- Web of Science ID : WOS:000321219200011